- Andy Lau as Senior Inspector Lau Kin-ming (劉健明), a former triad mole in the police force who tries to cover his past and remain as a cop
- Edison Chen as young Lau Kin-ming
- Tony Leung as Chan Wing-yan (陳永仁), an undercover cop. He was killed in the first film.
- Shawn Yue as young Chan Wing-yan
- Leon Lai as Superintendent Yeung Kam-wing (楊錦榮), Lau's rival in the police force
- Eddie Li as young Yeung Kam-wing
- Chen Daoming as Shen Cheng "Shadow" (沈澄), a Mainland Chinese triad boss who is actually an undercover cop
- Kelly Chen as Dr. Lee Sum-yee (李心兒), Chan's therapist and love interest
- Anthony Wong as Superintendent Wong Chi-shing (黃志誠), Chan's superior. He was killed by Hon Sam's henchmen in the first film.
- Eric Tsang as Hon Sam (韓琛), the triad boss. He was killed by Lau in the first film.
- Chapman To as Tsui Wai-keung / "Crazy Keung" (徐偉強 / 傻強), Hon's henchman. He was killed in the first film.
- Berg Ng as Inspector Cheung (張SIR)
- Wan Chi-keung as Officer Leung (梁SIR)
- Gordon Lam as Inspector Lam Kwok-ping / "Inspector B (Billy)" (林國平 / 大B), the triad mole who killed Chan in the first film. He was shot by Lau after revealing his true identity.
- Sammi Cheng as Mary, Lau's wife. A younger Mary was seen in the last part of the second film in the police station scene.
- Carina Lau as Mary, Hon Sam's wife whom Lau had a crush on. She was mowed down by a car in the second film.
- Huang Zhizhong as Shen Liang (沈亮)
- Waise Lee as Sergeant Chan Chun (陳俊)
Read more about this topic: Infernal Affairs III
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