- Seth Rogen as Britt Reid / The Green Hornet: A wealthy newspaper publisher who is secretly the masked crimefighter The Green Hornet.
- Jay Chou as Kato: A personal mechanic and martial arts expert who becomes the Green Hornet's valet and sidekick.
- Christoph Waltz as Benjamin Chudnofsky: A paranoid Russian gangster who plans to join all of the crime families of Los Angeles together to organize a "super-mafia."
- Cameron Diaz as Lenore "Casey" Case: The love interest of Reid and Kato. She is also Reid's secretary for The Daily Sentinel.
- Tom Wilkinson as James Reid: Britt's stern, wealthy father and a successful newspaper publisher.
- David Harbour as District Attorney Frank Scanlon: Scanlon is an ally of Benjamin Chudnofsky who bribed town officials into downplaying the city's level of crime in order to help his career.
- Edward James Olmos as Mike Axford, managing editor of The Daily Sentinel
- Jamie Harris as Popeye
- Chad Coleman as Chili
- Edward Furlong as Tupper: A meth producer
- Analeigh Tipton as Ana Lee
- Reuben Langdon as Crackhead
- Jerry Trimble as Chudnofsky's man
- James Franco as Danny "Crystal" Clear (uncredited), a young meth dealer and rival of Chudnofsky who is killed by a remote-activated briefcase bomb left upon Chudnofsky's departure that destroyed his nightclub.
Read more about this topic: The Green Hornet (2011 Film)
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“The statue of Freedom has not been cast yet, the furnace is hot, we can all still burn our fingers.”
—Georg Büchner (18131837)
“Has he all that the world loves and admires and covets?he must cast behind him their admiration, and afflict them by faithfulness to his truth, and become a byword and a hissing.”
—Ralph Waldo Emerson (18031882)